Interesting pairing this one, but I have to go for Loveless of course. While it's nearly impossible to compare both of them musically they did both have a significant impact on alternative music at the time, Nevermind more so in the mainstream, and also on myself. These days Loveless is far more interesting to me musically as I love getting lost in a nice big sea of sound, while ten years ago Nevermind would be the obvious choice for me as I would definitely prefer the youthful intensity and angst-ridden lyrics. Comparing the two of them now Loveless is way ahead of Nevermind in originality, creativity and consistency, while Nevermind only gets one up on Loveless in terms of energy.
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