I honestly would go with Combat Rock, even though it's not the most popular choice. It's their most complete and unified work, closely followed by their debut, but the aggregate quality isn't as high on that one as on Combat Rock, IMO. London Calling and Sandinista! have their best music, but those both have loads of filler and even bad songs and would have been much better if condensed to single discs.
Not much to say about Give Em' Enough Rope. It's just there. I haven't even bothered listening to Cut the Crap out of the assumption that it's as bad as everyone says.
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