I'll make a few more suggestions since this list is somewhat woefully incomplete:
Miles Davis - Bitches Brew (more or less the first fusion album)
i'll second Ornette Coleman - Shape of Jazz to Come
Talk Talk - Laughing Stock (laid the foundation for post-rock)
Whitehouse - Erector (first power electronics album)
Throbbing Gristle - Second Annual Report of Throbbing Gristle (arguably first industrial album?)
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