Booker T. & The MG's; Time Is Tight. The rest of their tracks are agreeable enough, but this one is transcendent.
A bit more controversial; Jimi Hendrix, Axis (Bold As Love). Amazing, mindblowing song. No other Hendrix track even comes close for me.
Even more controversial (?); Nirvana, Something In The Way. Love this song! Most every other Nirvana song is pretty dull.
...but a relatively "minor" artist? Has to be Vienna, by Ultravox. Midge Ure's a complete hack and Ultravox is basically a less commerically successful version of Duran Duran (shudder), but Vienna is one of those perfect pop songs.
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"This sure doesn't look like 'Crazy Ernie's Amazing Emporium of Total Bargain Madness!'"
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