Off the top of my head:
Torture Garden - Naked City(And there is a LOT of weird, and weirder, Zorn beyond that but Torture Garden is more significant than most of the really weird ones.)
Eskimo - Residents
I think the First Secret Chiefs album was quite weird even if the later ones are more composed
Helter Stupid - Negativland, not as good as Escape from Noise but of what I've heard, weirder
Requiem - Gyorgy Ligeti(Albeit, not technically an "album")
Almost anything by Boredoms, the earlier the weirder usually. I guess Pop Tatari is pretty weird.
I guess, of the listed, Eskimo would be the "weirdest".
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