I voted "Hi Baku Sho" as the most evocative of a post-apocalyptic soundtrack. I could perfectly see that song being played in the minutes directly following the aftermath of Hiroshima and Nagasaki.
Another close choice was the Portishead song, though I decided that it was more depressing in general and not necessarily post-apocalyptic.
Oh, and "Diabolique" would have been a fantastic song if the f***ing looped clip of "diabolical laughter" didn't ruin it. I mean, a couple times would have been OK, but it was so omnipresent that it interfered with the rest of the song.
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